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REVIEW
Contents Vol 66(5)

Critical Review of Water Radiolysis Processes, Dissociation Products, and Possible Impacts on the Local Environment: A Geochemist’s Perspective

Soumya Das
+ Author Affiliations
- Author Affiliations

Department of Geological Sciences, University of Saskatchewan, 114 Science Place, Saskatoon, SK S7N 5E2, Canada. Email: sod671@campus.usask.ca




Dr. Das completed his B.Sc. (1995) and M.Sc. (1997) degrees in Geology at the University of Calcutta, India. He then worked as a Research Fellow doing mineral exploration at Bengal Engineering College, India until 1999. He received a Masters degree in Geology (Petrology/Mineral Chemistry) in 2002 from the University of Akron, USA, followed by a Ph.D. in Aqueous Geochemistry in 2007 from Western Michigan University, USA. In recent years, he has worked as a Post-doctoral Associate at Rutgers University, USA (2007–2008) and as a Professional Research Associate at the University of Saskatchewan, Canada (2008–present) in Aqueous/Environmental Geochemistry.

Australian Journal of Chemistry 66(5) 522-529 https://doi.org/10.1071/CH13012
Submitted: 9 November 2012  Accepted: 16 February 2013   Published: 3 April 2013

Abstract

Radiolysis of water is the process whereby water dissociates due to various types of ionizing radiation (α, β, and γ) into hydrogen and hydroxide radicals (instead of hydrogen and hydroxide ions as in ionization). During radiolysis, water breaks down to highly reactive radicals such as •OH, •H, eaq–, HO2, and O2–• and molecular species such as H2, O2, and H2O2. Yields of these dissociation products are largely dependent on factors including the type of radiation, vapour pressure of the system, and linear energy transfer. These dissociated radicals are highly reactive and can affect the local environment by changing redox conditions and, in turn, inducing and enhancing metal mobility in the environment. This article reviews the process of water radiolysis, dissociation products, and possible effects on the environment.


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