Chemical and dispersal characteristics of particulate emissions from forest fires in Siberia
Y. N. Samsonov A E , V. A. Ivanov B , D. J. McRae C and S. P. Baker DA Institute of Chemical Kinetics and Combustion, 630090 Novosibirsk, Russia.
B Siberian State Technological University, Forest Institute, 660036 Krasnoyarsk, Russia.
C Canadian Forest Service, 1219 Queen Street East, Sault Ste Marie, ON, P6A 2E5, Canada.
D Rocky Mountain Research Station, USDA Forest Service, Missoula, MT 59807, USA.
E Corresponding author. Email: samsonov@kinetics.nsc.ru
International Journal of Wildland Fire 21(7) 818-827 https://doi.org/10.1071/WF11038
Submitted: 14 March 2011 Accepted: 12 February 2012 Published: 11 July 2012
Abstract
Approximately 20 experimental fires were conducted on forest plots of 1–4 ha each in 2000–07 in two types of boreal forests in central Siberia, and 18 on 6 × 12-m plots in 2008–10. These experiments were designed to mimic wildfires under similar burning conditions. The fires were conducted in prescribed conditions including full documentation on pre-fire weather, pre-fire and post-fire forest fuels, fire intensities, and other biological, physical and chemical parameters. The amount of particulate matter emitted during a typical fire averaged 0.6 t ha–1 and ranged within 0.2–1.0 t ha–1 depending on burning conditions. Particulates accounted for ~1–7% of the total mass of the consumed biomass during a typical forest fire (10–30 t ha–1 based on our data from 2000–07). Most of the particulate matter consists of organic substances, 77% on average, with a range of 70–90%. Elemental carbon averaged 8%, with a range of 2–18%. Trace element compositions and amounts of particulates indicate that there was no actual difference in the element emissions sampled from the fires conducted in the two forest types (6–8% in larch forest and 8% in pine forest). Most of the particulate matter, 90–95%, consists of submicrometre and near-micrometre particles ~0.1–5 μm in diameter.
Additional keywords: black carbon, chemical composition, elemental carbon, organic carbon, smoke particulate.
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