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RESEARCH ARTICLE
Contents Vol 70(3)

Two 3D ZnII Metal–Organic Frameworks with 3- and 8-Fold Interpenetration: Syntheses, Structures, Photodegradation, and Photoluminescent Properties

Chuan-Bin Fan A , Xiang-Min Meng A , Yu-Hua Fan A , Zi-Ao Zong A , Xiao-Yin Zhang A and Cai-Feng Bi A B
+ Author Affiliations
- Author Affiliations

A Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao, Shandong 266100, China.

B Corresponding author. Email: bicaifeng301@163.com

Australian Journal of Chemistry 70(3) 314-321 https://doi.org/10.1071/CH16368
Submitted: 21 June 2016  Accepted: 1 September 2016   Published: 21 September 2016

Abstract

Two novel coordination polymers, namely {[Zn(sbdc)(bmib)]·0.4H2O}n (1) and {[Zn(sbdc)(bibd)]·DMF}n (2) (H2sbdc = 4,4′-stilbenedicarboxylic, bmib = 1,4-bis(2-methylimidazol-1-yl)butane, bibd = 1,1′-(1,4-butanediyl)bis(imidazole), DMF = N,N-dimethylformamide), have been acquired under solvothermal conditions, and have been characterised by elemental analysis, infrared spectra, thermogravimetric analysis, and single-crystal X-ray diffraction (XRD). Single-crystal XRD analysis reveals that 1 shows eight-fold interpenetrating 3D frameworks with a four-connected (66) sqc6 topology and 2 displays four-connected three-fold interpenetrating 3D frameworks. The flexible N-donor ligands play an important role in the construction of the final topological structures for 1 and 2. Furthermore, 1 and 2 exhibit good photodegradation capability and photoluminescence properties.


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