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Australian Journal of Chemistry Australian Journal of Chemistry Society
An international journal for chemical science
RESEARCH ARTICLE

Grand ensemble Monte Carlo study of crystallization in sub-monolayer adsorption at a solid vapour interface

JE Lane and TH Spurling

Australian Journal of Chemistry 31(5) 933 - 942
Published: 1978

Abstract

A grand ensemble Monte Carlo procedure is used to examine the thermodynamic properties of a crystal-like layer of krypton adsorbed at sub-monolayer coverages on graphite at 90.12 K. The effect of the periodic boundary conditions on these properties is discussed and used to develop a thermodynamically consistent iterative procedure to estimate the transition pressure and thereby fix the adsorption isotherm.

https://doi.org/10.1071/CH9780933

© CSIRO 1978

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